In this particular case you could use a combination of x86 SHR and RCR instructions:
; a0 - bits 0-31 of a[i]
; a1 - bits 32-63 of a[i]
; a2 - bits 64-95 of a[i]
; a3 - bits 96-127 of a[i]
mov eax, a0
mov ebx, a1
mov ecx, a2
mov ecx, a3
shr eax, 1
rcr ebx, 1
rcr ecx, 1
rcr edx, 1
; b0 - bits 0-31 of b[i] := a[i] >> 1
; b1 - bits 32-63 of b[i] := a[i] >> 1
; b2 - bits 64-95 of b[i] := a[i] >> 1
; b3 - bits 96-127 of b[i] := a[i] >> 1
mov b0, eax
mov b1, ebx
mov b2, ecx
mov b3, edx
shr eax, 1
rcr ebx, 1
rcr ecx, 1
rcr edx, 1
; c0 - bits 0-31 of c[i] := a[i] >> 2 = b[i] >> 1
; c1 - bits 32-63 of c[i] := a[i] >> 2 = b[i] >> 1
; c2 - bits 64-95 of c[i] := a[i] >> 2 = b[i] >> 1
; c3 - bits 96-127 of c[i] := a[i] >> 2 = b[i] >> 1
mov c0, eax
mov c1, ebx
mov c2, ecx
mov c3, edx
If your target is x86-64 this simplifies to:
; a0 - bits 0-63 of a[i]
; a1 - bits 64-127 of a[i]
mov rax, a0
mov rbx, a1
shr rax, 1
rcr rbx, 1
; b0 - bits 0-63 of b[i] := a[i] >> 1
; b1 - bits 64-127 of b[i] := a[i] >> 1
mov b0, rax
mov b1, rbx
shr rax, 1
rcr rbx, 1
; c0 - bits 0-63 of c[i] := a[i] >> 2 = b[i] >> 1
; c1 - bits 64-127 of c[i] := a[i] >> 2 = b[i] >> 1
mov c0, rax
mov c1, rbx
Update: corrected typos in 64-bit version